TY - JOUR
T1 - Activated carbon preparation from biomass feedstock
T2 - Clean production and carbon dioxide adsorption
AU - Ahmed, Mohammad Boshir
AU - Hasan Johir, Md Abu
AU - Zhou, John L.
AU - Ngo, Huu Hao
AU - Nghiem, Long Duc
AU - Richardson, Christopher
AU - Moni, Mohammad Ali
AU - Bryant, Macguire R.
N1 - Publisher Copyright:
© 2019 Elsevier Ltd
PY - 2019/7/10
Y1 - 2019/7/10
N2 - The current methods used for the production of activated carbon (AC) are often chemical and energy intensive and produce significant amount of chemical waste. Thus, clean production of AC is important to reduce its overall production cost and to limit the adverse effect on the environment. Therefore, the main aim of this study is to develop a clean method for AC production from woody biomass with low chemical consumption. Herein, this study reports a facile strategy for reducing chemical usages in the production of high-performance AC, by introducing a crucial pre-pyrolysis step before chemical activation of biomass. The ACs prepared were characterised using scanning electron microscopy, Fourier transform infrared spectroscopy, nitrogen and carbon dioxide gas adsorption measurements. All these characterisations indicated that produced ACs have similar physicochemical properties. The strategy reduced chemical use by 70% and produced high-performance ultra-microporous ACs with excellent carbon dioxide adsorption capacity (4.22–5.44 mmol m −2 ). The facile pre-pyrolysis method is recommended for further research as a cleaner activated carbon preparation method from biomass feedstock.
AB - The current methods used for the production of activated carbon (AC) are often chemical and energy intensive and produce significant amount of chemical waste. Thus, clean production of AC is important to reduce its overall production cost and to limit the adverse effect on the environment. Therefore, the main aim of this study is to develop a clean method for AC production from woody biomass with low chemical consumption. Herein, this study reports a facile strategy for reducing chemical usages in the production of high-performance AC, by introducing a crucial pre-pyrolysis step before chemical activation of biomass. The ACs prepared were characterised using scanning electron microscopy, Fourier transform infrared spectroscopy, nitrogen and carbon dioxide gas adsorption measurements. All these characterisations indicated that produced ACs have similar physicochemical properties. The strategy reduced chemical use by 70% and produced high-performance ultra-microporous ACs with excellent carbon dioxide adsorption capacity (4.22–5.44 mmol m −2 ). The facile pre-pyrolysis method is recommended for further research as a cleaner activated carbon preparation method from biomass feedstock.
KW - Activated carbon
KW - Biomass
KW - Chemical activation
KW - CO adsorption
KW - Surface area
UR - http://www.scopus.com/inward/record.url?scp=85064223813&partnerID=8YFLogxK
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U2 - 10.1016/j.jclepro.2019.03.342
DO - 10.1016/j.jclepro.2019.03.342
M3 - Article
AN - SCOPUS:85064223813
SN - 0959-6526
VL - 225
SP - 405
EP - 413
JO - Journal of Cleaner Production
JF - Journal of Cleaner Production
ER -